The Journal of Chemical Physics
We investigate spectral diffusion decay using a model for solids that consists of two‐level‐systems (TLSs) interacting via strain fields. For the case when the rate of TLS flips vanishes, we find algebraic decay of correlation functions of the local field. We show that properties of equilibrium fluctuations are in agreement with the hierarchical picture proposed by Basché and Moerner: TLSs far away produce fast fluctuations that are small in magnitude, and close TLSs produce large fluctuations that are less frequent.
Zürcher, Ulrich, "A Stochastic Theory of Inhomogeneously Broadened Linewidths in Solids" (1995). Physics Faculty Publications. 279.
© 1995 American Institute of Physics.